Magnetic polarization of the americium J=0 ground state in AmFe(2).

نویسندگان

  • N Magnani
  • R Caciuffo
  • F Wilhelm
  • E Colineau
  • R Eloirdi
  • J-C Griveau
  • J Rusz
  • P M Oppeneer
  • A Rogalev
  • G H Lander
چکیده

Trivalent americium has a nonmagnetic (J=0) ground state arising from the cancellation of the orbital and spin moments. However, magnetism can be induced by a large molecular field if Am^{3+} is embedded in a ferromagnetic matrix. Using the technique of x-ray magnetic circular dichroism, we show that this is the case in AmFe_{2}. Since ⟨J_{z}⟩=0, the spin component is exactly twice as large as the orbital one, the total Am moment is opposite to that of Fe, and the magnetic dipole operator ⟨T_{z}⟩ can be determined directly; we discuss the progression of the latter across the actinide series.

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عنوان ژورنال:
  • Physical review letters

دوره 114 9  شماره 

صفحات  -

تاریخ انتشار 2015